CompuServe Thread

#Hydrogen Sulfide danger

18 messages in this thread
#152076From: Michael SternbergNov 2, 1994 11:09 PM
Doug- Olfactory paralysis from H2S inhalation is a fact. I will endeavor to find a medical description of the mechanism involved. Regrettably, work has severely impacted on my free time lately…seems like always…and I haven't been able to keyboard the H2S Toxicity data I mentioned a while back. Instead, I will be happy to photocopy it ( about 4 pages ) and mail to anyone who wants a copy. Since I don't have it sitting here at home, I won't try to list specific levels (ppm) at which various physiological effects begin and possibly be in error. Regards- Michael
#152234From: Jim YahrNov 3, 1994 9:55 PM
Michael, PMFJI I've been lurking this forum for a couple of months, but this seems like a good place to say something. I work around the H2S somewhat regularly, have taught the safety course required by law for oil field workers, and just completed my annual safety certification to work in the oil fields in an H2S environment, here are the ANSI 23Z-1972 standards: 0.0002 percent (2ppm) Obvious odor 0.001 percent (10ppm) Beginning eye irritation (OSHA 8 hour max exposure) 0.0015 percent (15 ppm) STEL (Short Term Exposure Limit) 0.01 percent (100 ppm) Coughing, eye irritation, loss of smell in 2-5min 0.02 percent (200 ppm) marked conjunctivitis, respiratory tract irritation in 1 hour 0.05 percent (500 ppm) loss of conciousness, possible death in 30 min-1hr 0.07 percent (700 ppm) Rapid unconciousness, breathing will stop and death will occur if not promptly rescued 0.10 percent (1000 ppm) Immediate unconciousness, early cessation of breathing and death within minutes. Death may occur even if moved to fresh air at once. This is dangerous stuff. The only gas more lethal (other than some specialized chem warfare stuff) is hydrogen cyanide (HCN). Additionally mixtures of 4.3 to 46 pervent volume in air is explosive, it burns to form sulfur dioxide (another poisonous, but less toxic gas), and is water soluable (4 parts H2S to 1 part water at 32 degrees F).
#152291From: SyndesisNov 4, 1994 9:03 AM
I think it's tough for people to understand even straightforward numbers like relative risk of dying in a car versus an airplane… Can you place those numbers in perspective? For example, what's a common way to produce H2S, and how much of those reactants would produce enough gas in a closed 10 x 10 room in order to reach 0.05 percent? What's a common reaction that produces the whiff of obvious odor?
#152536From: Michael SternbergNov 5, 1994 11:42 PM
John- The values Jim cited are volumetric basis. A 10x10x8 ft room contains 800 cubic feet. You would have to have 0.4 ft^3 or ~11.5 liters of 100% H2S to reach a 500 ppm concentration. This is extremely unlikely in most circumstances at home, but is entirely possible in some mines lacking ventilation. A far greater risk to rockhounds is entering areas of low oxygen concentration. Hypoxic conditions can occur anywhere insufficient air circulation combines with oxygen hungry materials such as sulfide or telluride ore bodies or high concentrations of organic material. Several years ago, three crew members of a Tuna fishing boat died from both H2S exposure and hypoxia when they lost refrigeration of the fish hold and the tuna began to rot. They attempted to remove the decomposing tuna and died when they entered the confined space. Death was immediate. Oil and natural gas Refining necessarily produce H2S in desulphering crude oil or gas. H2S naturally occurs in oil and gas fields. Many natural gas plants desulfur the natural gas using Claus process sulfur recovery. If you ever fly over Alberta, north of Calgary are huge, and I mean huge!, blocks of sulfur recovered from natural gas. Most refineries produce H2S as a byproduct from crude distallation, catalytic cracking units, hydrotreating and decoking (among others). This H2S is usually converted to elemental sulfur using Sulfur Recovery units. We also operate a Sulfur Recovery Unit and produce about 20 Tons/day of molten sulfur. Someday, I intend to play around with controlled cooling of molten sulfur to try to produce large sulfur crystals. However, sulfur is *really* peculiar. Unlike most liquids, molten sulfur viscosity increases with temperature to become a tarry substance, further heating then results in a drop in viscosity. This is due to the bonding nature of sulfur. It exists as various species, S2, S3, S4, S6, S8 and polyermic S. Forming sulfur crystals is very dependent on initial temperature and rate of cooling. No nearly as simple as making "rock" candy. Michael
#152589From: SyndesisNov 6, 1994 11:59 AM
OK, I'll stay away from rotting tuna. 🙂
#152663From: Tom LeCompte-SysopNov 6, 1994 7:36 PM
My experiment uses large quantities of Argon-Ethane gas. One of the worst contaminents is H2S, and every once in a while we get a truck full of it. I always wondered why H2S is associated with ethane. Now I know – thanks!
#152683From: SyndesisNov 6, 1994 8:56 PM
How large are those "blocks of sulfur"?
#153026From: Michael SternbergNov 9, 1994 9:12 PM
John – I will have to make a phone call to find out. I do not want to exaggerate the size, nor understate it. For now, I can definitely say that from the air, they appeared to cover about 2-3 acres and were about 40 feet high. Will get the facts. Michael
#152742From: Jim YahrNov 7, 1994 1:31 PM
John, The most common method of producing H2S is the decay of biological material. Hence the name "rotten egg gas". Your nose can detect down to 0.13 ppm. That's roughly 1/8 of 100 ppm or if you want a different comparison, about 1/6 of an inch out of 15.5 miles. Around the home, H2S can be present in sewers, rotten garbage, compost piles, and similar settings. The most common source is probably by "passing gas". Entire oil drilling rigs have been cleared here in Texas because one of the roughnecks ate too much Mexican food and "broke wind" near a sensor. (The alarms are set to trigger at 10 ppm) I can't really think of a common reaction that would fill a 10X10 room in a houshold setting. Mixing sulfuric acid (present in some tile cleaners), with ammonia could produce H2S. I doubt that lethal concentrations could build up in a home under normal circumstances, but pouring sulfuric acid down the drain in an older home (with iron sewer pipe.) might. In laboratories, reactions of sulfuric acid w/ other sulfur containing compounds can produce H2S. I've heard of High Schools were one of the kids decided to make a stink bomb with FeS and H2SO4 and the entire building was evacuated. Pouring H2SO4 down the sewers might, and muriatic acid (used for etching tile, and in swimming pools), could react with sulfur containing compunds to produce the same result. I'll think some more about it. Jim
#152857From: SyndesisNov 8, 1994 10:14 AM
H2S is only produced by anaerobic reactions, right? A well-maintained compost pile shouldn't smell like that, but that's a topic for the gardening forum. 🙂 As for the 10 x 10 room, I meant what sort of household reaction would produce dangerous levels of H2S. As you said, there are certainly situations where household chemicals can do it. As for human-produced H2S, are you saying that the level could approach 10 ppm?
#153019From: Jim YahrNov 9, 1994 8:33 PM
>>As for human-produced H2S, are you saying that the level could approach 10 ppm? Yes, The situations I know about, the sensors that triggered, and the people that triggered them were in the cellar, which is a confined spave below the drilling rig, where the casin on the well comes out of the ground. According to OSHA regs you can work in a max of 10ppm for 8 hours a day, 40 hrs. per week with no additional protection. >>H2S is only produced by anaerobic reactions, right? Right.
#153028From: Michael SternbergNov 9, 1994 9:13 PM
Actually, human flatulence consists primarily of methane with lesser levels of mercaptans and much lower levels of H2S. Mercaptans are sulfur-bearing hydrocarbons that are more often associated with skunk odor, and are used to odorize natural gas and LPG for domestic consumption. As an aside, intestinal gas has resulted in surgery room explosions, albeit rarely. In our house, with 4 males, explosion is the least of our worries, and may answer your question about how to fill a 10×10 room. <g>
#153040From: SyndesisNov 9, 1994 10:26 PM
Hmm, flatulence trivia… Japanese children have flashcards to help them learn the 50-or-so basic phonetic sounds of their syllabary. One is "fu," and the flashcard usually shows a fat naked guy (think of a Japanese construction worker in loincloth, or a sumo wrestler) with comic-book-like "wind lines" near his behind. I see to remember that a variety of mercaptan is listed in the Guinness Book of World Records, as a smell recognizable at the lowest levels, which makes it "smelliest" in some sense.
#153027From: Michael SternbergNov 9, 1994 9:12 PM
Jim- don't forget about the dangers of setting up a Popeil Kitchen Refinery (not available in stores). <G>
#152535From: Michael SternbergNov 5, 1994 11:42 PM
Jim- Thanks for the summary of H2S toxicology. It is what I have intended to post for some time, but haven't somehow coordinated (wonder if a busy schedule is any factor). I work in a sulfuric acid plant that processes up to 84 tons of H2S per day. In 37 years, we have had zero incidents involving plant personnel. Although 28 years ago, we did experience a significant leak in a pipeline that did kill a rabbit and three birds. Most forum members will not be exposed to substantial risk in their normal activities, however there are some circumstances in the field where significant concentrations of H2S can occur: Sulfide zones of ore deposits evolve H2S which is slighty heavier than air. Localized areas of fatal concentrations can occur. Coal deposits and some carbonaceous shales are another potential exposure. Hydrothermal zones near active volcanoes or other geothermal structures. If sulfur deposits are present, you can bet H2S was the source. SO2 (sulfur dioxide) is less lethal than H2S at similar concentrations, yet its PEL (permitted exposure limit) is 5 ppm or half the allowable exposure limit of H2S. SO2 has such an irritating effect on mucosal membranes that rarely will an individual chose to remain in exposure for long, and certainly it warns you well before you hit a lethal level. The toxicity of H2S is due to its chemical binding with haemoglobin forming methaemoglobin. The oxygen carrying capacity of the circulatory system is rapidly and significantly diminished. Fortunately, the effects are relatively quick to reverse, provided the victim is removed to an H2S free area. There is a marvelous training film on H2S that demonstrates the effect of H2S exposure and subsequent recovery on a rat. Regards- Michael
#152634From: Doug MitchellNov 6, 1994 4:18 PM
Hi, Jim– Welcome to the forum/section! Thanks for the info. I am pleased to hear there is a lot of watering of the eyes and other symptoms to drive one away before the danger gets severe, provided one does not generate too much H2S too fast. It suggests to me I am not being crazy when I heat a small specimen in my apartment, though I will continue to make sure the fan is on and the windows open when I do such things. Anyone care to figure roughly how big a specimen of sulfide ore would have to be to endanger one's life before one could be driven out of a room by the smell and irritation? Let's say 0 to 500 ppm in a minute is too fast, or 11 liters/minute is too fast (see Michael's post in this topic). How much sulfide ore can make 11 liters of H2S gas (at room temperature/pressure)? Without a ready supply of acid, and assuming there is not a lot of bisulfide in the ore, it may be quite large. Anyway, dripping a bit of HCl on a specimen and smelling the bubbles for H2S cannot be producing enough unless they are _very large_ bubbles. –Doug
#153029From: Michael SternbergNov 9, 1994 9:13 PM
Remember–from Jim's table– 1000ppm will cause immediate unconciousness. 1000ppm is equivalent to 1 milliliter(100%H2S)/liter. One shallow breath is approximately 1 liter. So all that needs to be evolved near your snout is 1 to 2 mls of H2S to put you down. A pound of sulfide ore in acid sould provide more than that I think. Haven't done the stoichiometry yet. Michae
#153048From: Doug MitchellNov 9, 1994 10:57 PM
Hi, Michael– I knew there was a reason I only heat small grains of mineral, and only put a drop or two of acid on a specimen (besides destroying too much of the specimen, that is). 🙂 Even that pound in acid might not generate that ml of H2S fast enough to knock me over before it disperses a bit (assuming I do not heat the acid), but I am not ready to bet my life on it. –Doug